Temporal change in fallout 137Cs in terrestrial and aquatic systems:  A whole ecosystem approach

Smith, James T.; Fesenko, Serguei V.; Howard, Brenda J. ORCID: https://orcid.org/0000-0002-9698-9524; Horrill, A. David; Sanzharova, Natalya I.; Alexakhin, Roudolf M.; Elder, David G.; Naylor, Christopher. 1999 Temporal change in fallout 137Cs in terrestrial and aquatic systems:  A whole ecosystem approach. Environmental Science & Technology, 33 (1). 49-54. https://doi.org/10.1021/es980670t

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Abstract/Summary

During the years after a nuclear accident, the bioavailability and environmental mobility of radiocesium declines markedly, resulting in large changes in contamination of foodstuffs, vegetation, and surface waters. Predicting such changes is crucial to the determination of potential doses to affected populations and therefore to the implementation of radiological countermeasures. We have analyzed 77 data sets of radiocesium (137Cs) activity concentrations in milk, vegetation, and surface waters after the Chernobyl accident. Our results show that the rate of decline in 137Cs during the years after Chernobyl is remarkably consistent in all three ecosystem components, having a mean effective half-life,Teff2 years. By comparing changes in 137Cs availability with rates of diffusion of 40K (a close analogue) into the lattice of an illitic clay (1)we have, for the first time, directly linked changes in the environmental availability of 137Cs to fixation processes at a mechanistic level. These changes are consistent with declines in the exchangeable fraction of 137Cs in soils (2, 3).

Item Type:	Publication - Article
Digital Object Identifier (DOI):	https://doi.org/10.1021/es980670t
Programmes:	CEH Programmes pre-2009 publications > Other
UKCEH and CEH Sections/Science Areas:	_ Pre-2000 sections
ISSN:	0013-936X
Additional Keywords:	radioecology
NORA Subject Terms:	Ecology and Environment
Date made live:	24 May 2012 09:28 +0 (UTC)
URI:	https://nora.nerc.ac.uk/id/eprint/17772

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