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Processes of ammonia air-surface exchange in a fertilized corn canopy

Walker, J. T.; Bash, J. O.; Jones, M.; Nemitz, E.; Robarge, W. P.. 2009 Processes of ammonia air-surface exchange in a fertilized corn canopy. Eos, Transactions, American Geophysical Union, 90 (52 Fall Meet. Su), Abstract A51E-0161.

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Abstract/Summary

Processes of ammonia (NH3) air-surface exchange in fertilized crops include bi-directional flux (emission or deposition) from the soil, surface litter, leaf stomatal cavity, and leaf cuticle. These component fluxes establish the net exchange between the canopy and atmosphere. We conducted an experiment in the summer of 2007 in eastern North Carolina to quantify the net flux of NH3 from a fertilized corn canopy over the course of the growing season. A primary objective was to examine the relative importance of soil vs. foliage exchange pathways with respect to net canopy-scale fluxes. Continuous wet rotating denuder and photoacoustic spectroscopic NH3 measurement methods were configured in a gradient mode to measure canopy-scale fluxes using the modified Bowen-ratio technique. In-canopy source-sink relationships were examined by inverse modeling of NH3 concentration, temperature, and turbulence profiles. Additionally, measurements of NH4+ and H+ in the soil solution, leaf apoplast, and leaf surface water were used in combination with resistance modeling to examine the relationships between net canopy-scale fluxes and soil, stomatal, and cuticular exchange pathways. Measurement and modeling results are presented and the relevance of this work to national NH3 emission inventories and regional air quality modeling is discussed.

Item Type: Publication - Article
Programmes: CEH Topics & Objectives 2009 - 2012 > Biogeochemistry > BGC Topic 2 - Biogeochemistry and Climate System Processes > BGC - 2.1 - Quantify & model processes that control the emission, fate and bioavailability of pollutants
CEH Topics & Objectives 2009 - 2012 > Biogeochemistry > BGC Topic 1 - Monitoring and Interpretation of Biogeochemical and Climate Changes > BGC - 1.4 - Develop innovative, effective methods for monitoring fluxes, exposure and effects
CEH Topics & Objectives 2009 - 2012 > Biogeochemistry > BGC Topic 1 - Monitoring and Interpretation of Biogeochemical and Climate Changes > BGC - 1.1 - Monitor concentrations, fluxes, physico-chemical forms of current and emerging pollutants ...
CEH Sections: Billett (to November 2013)
ISSN: 0096-3941
Additional Information. Not used in RCUK Gateway to Research.: Abstract only
Additional Keywords: agricultural systems, biogeochemical cycles, biosphere/atmosphere interactions
NORA Subject Terms: Atmospheric Sciences
Date made live: 28 Apr 2010 10:03
URI: http://nora.nerc.ac.uk/id/eprint/9345

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